Ageing Resistance of Bituminous Binder Modified with Propitious Antioxidant

Document Type : Research Papers

Authors

1 Assistant Professor, Department of Civil Engineering, National Institute of Technology Patna, Bihar, India.

2 Professor, Department of Civil Engineering, National Institute of Technology Patna, Bihar, India.

3 M.Tech., Department of Civil Engineering, National Institute of Technology Patna, Bihar, India.

Abstract

Bituminous mixes are prepared with aggregates, filler and bitumen as binder. Ageing of bitumen due to oxidation reduces the durability of such mixes. Various research efforts are therefore put in to decrease the ageing potential of binders and use of anti-oxidants has shown substantial success. In this research, Irganox 1010 has been identified as an anti-oxidant which has been found to be economical and yet of limited use in the field of pavement engineering. Various physical and rheological tests were conducted to determine the influence of Irganox 1010 on short-termed as well as long termed aged binders and results were analyzed. Softening Point Index (SPI) and Viscosity Ageing Index (VAI) were determined to understand the influence of Irganox 1010 on bituminous mixes. It was observed that Irganox 1010 significantly reduce ageing potential with usage of 0.6% by weight of bitumen. It has been found to be cost-effective due requirement of small quantities and being of comparatively lesser cost. This material has the potential of large scale usage to increase durability of bituminous mixes.

Keywords


Apeagyei, A.K. (2011). “Laboratory evaluation of antioxidants for asphalt binders”, Construction and Building Materials, 25, 47-53, https://doi.org/10.1016/j.conbuildmat.2010.06.058.
Alae, M., Zhao, Y. and Leng, Z. (2021). “Effects of ageing, temperature and frequency-dependent properties of asphalt concrete on top-down cracking”, Road Material Pavement Design, 22(10), 2289-2309, https://doi.org/10.1080/14680629.2020.1753099.
Al-Mansob, R.A., Ismail, A., Md-Yusoff, N.I., Albrka, SI., Azhari, C.H. and Karim, M.R. (2016). “Rheological characteristics of unaged and aged epoxidised natural rubber modified asphalt”, Construction and Building Materials, 102, 190-199, https://doi.org/10.1016/j.conbuildmat.2015.10.133.
Arafat, S., Kumarm N., Wasiuddinm, N.W., Owhem E.O. and Lynamm, J.G. (2019). “Sustainable lignin to enhance asphalt binder oxidative aging properties and mix properties”, Journal of Cleaner Production, 217, 456-468, https://doi.org/10.1016/j.jclepro.2019.01.238.
ASTM D5. (1997). Standard test method for penetration of bituminous materials, American Society for Testing and Materials, Conshohocken, Pennsylvania, USA.
ASTM D36. (1995). Standard test method for softening point of bitumen (Ring-and-Ball apparatus), American Society for Testing and Materials, Conshohocken, Pennsylvania, USA.
ASTM D-4402. (2000). Standard test method for viscosity determination of asphalt at elevated temperatures using a rotational viscometer, American Society for Testing and Materials, Conshohocken, Pennsylvania, USA.
ASTM D7175. (2015). Standard test method for determining the rheological properties of asphalt binder using a dynamic shear rheometer, ASTM International, West Conshohocken, Pennsylvania, USA.
ASTM D2872. (2019). Standard method of test for effect of heat and air on a moving film of asphalt (rolling thin-film oven test), ASTM International, West Conshohocken, PA, USA.
ASTM D6521. (2000). Standard practice for accelerated aging of asphalt binder using a Pressurized Aging Vessel (PAV), American Society for Testing and Materials, Conshohocken, Pennsylvania, USA.
Chakravarty, H. and Sinha, S. (2020). “Moisture damage of bituminous mixes and application of nanotechnology in its Prevention”, Journal of Materials in Civil Engineering, 32(8), 03120003, https://doi.org/10.1061/(ASCE)MT.1943-5533.0003293.
Cong, P., Wang, J., Li, K. and Chen, S. (2012). “Physical and rheological properties of asphalt binders containing various antiaging agents”, Fuel, 97, 678-684, https://doi.org/10.1016/j.fuel.2012.02.028.
Cong, P., Wang, X., Xu, P., Liu, J., He, R., Chen, S. (2013). “Investigation on properties of polymer modified asphalt containing various antiaging agents”, Polymer Degradation and Stability, 98, 2627-2634, https://doi.org/10.1016/j.polymdegradstab.2013.09.024.
Dickinson, E.J. (1980). “The hardening of Middle East petroleum asphalts in pavement surfacings, Proceedings of the Association of Asphalt Paving Technologists (AAPT), 49, 30-57.
Feng, Z., Yu, J., Zhang, H. and Kuang, D. (2011) “Preparation and properties of ageing resistant asphalt binder with various anti-ageing aadditives”, Applied Mechanics and Materials, 71-78, 1062-1067, https://doi.org/10.4028/www.scientific.net/AMM.71-78.1062.
Feng, Z., Rao, W., Chen, C., Tian, B., Li, X., Li, P. and Guo, Q. (2016). “Performance evaluation of bitumen modified with pyrolysis carbon black made from waste tyres”, Construction and Building Materials, 111, 495-501, https://doi.org/10.1016/j.conbuildmat.2016.02.143.
Feng, Z., Cai, F., Yao, D. and Li, X. (2021). “Aging properties of ultraviolet absorber/SBS modified bitumen based on FTIR analysis”, Construction and Building Materials, 273, Article 121713, https://doi.org/10.1016/j.conbuildmat.2020.121713.
Ji, X., Hou, Y., Zou, H., Chen, B. and Jiang. Y. (2020). “Study of surface microscopic properties of asphalt based on atomic force microscopy”, Construction and Building Materials, 242, Article 118025, https://doi.org/10.1016/j.conbuildmat.2020.118025.
Floody, A.C. and Thenoux, G. (2012). “Controlling asphalt aging by inclusion of byproducts from red wine industry”, Construction and Building Materials, 28, 616-623, https://doi.org/10.1016/j.conbuildmat.2011.08.092.
Fini, E.H., Buabeng, F.S., Abu-Lebdeh, T. and Awadallah,. F (2015). “Effect of introduction of furfural on asphalt binder ageing characteristics”, Road Materials and Pavement Design, 17(3), 638-657, https://doi.org/10.1080/14680629.2015.1108219.
Gokalp, I. and Uz, V.E. (2019). “Utilizing of waste vegetable cooking oil in bitumen: Zero tolerance aging approach”, Construction and Building Materials, 227, 116695, https://doi.org/10.1016/j.conbuildmat.2019.116695.
Gu, F., Ma, W., West, R.C., Taylor, A.J. and Zhang, Y. (2019). “Structural performance and sustainability assessment of cold central-plant and in-place recycled asphalt pavements: A case study”, Journal of Cleaner Production, 208, 1513-1523, https://doi.org/10.1016/j.jclepro.2018.10.222.
Hofko, B., Cannone Falchetto, A., Grenfell, J., Huber, L., Lu, X., Porot, L., Poulikakos, L.D. and You, Z. (2017). “Effect of short-term ageing temperature on bitumen properties”, Road Materials and Pavement Design, 18(sup2), 108-117, https://doi.org/10.1080/14680629.2017.1304268.
Hofko, B., Maschauer,, D., Steiner D., Mirwald, J. and Grothe, H. (2020). “Bitumen ageing, Impact of reactive oxygen species”, Case Study Construction Materials, 13, e00390, https://doi.org/10.1016/j.cscm.2020.e00390.
Lee, S.-J., Amirkhanian, S.N., Shatanawi, K. and Kim, K.W. (2008). “Short-term aging characterization of asphalt binders using gel permeation chromatography and selected superpave binder tests”, Construction and Building Materials, 22(11), 2220-2227, https://doi.org/10.1016/j.conbuildmat.2007.08.005.
Lian, H., Lin, J. and Yen, T.F. (1994). “Peptization studies of asphaltene and solubility parameter spectra”, Fuel, 73(3), 423-428, https://doi.org/10.1007/978-1-4899-0617-5_4.
Liu, X., Cao, F., Xiao, F. and Amirkhanian, S. (2018). “BBR and DSR testing of aging properties of polymer and polyphosphoric acid, modified asphalt binders”, Journal of Materials in Civil Engineering, 30(10), 04018249(1)-04018249(11), https://doi.org/10.1061/(ASCE)MT.1943-5533.0002440.
Luo, X., Gu, F., Zhang, Y., Lytton, R.L. and Birgisson, B. (2018). “Kinetics-based aging evaluation of in-service recycled asphalt pavement”, Journal of Cleaner Production, 200, 934-944, https://doi.org/10.1016/j.jclepro.2018.07.267.
Margaritis, A., Soenen, H., Fransen, E., Pipintakos, G., Jacobs, G. and Blom, J. (2020). “Identification of ageing state clusters of reclaimed asphalt binders using principal component analysis (PCA) and hierarchical cluster analysis (HCA) based on chemo-rheological parameters”, Construction and Building Materials, 244, 118276, https://doi.org/10.1016/j.conbuildmat.2020.118276.
Mirwald, J., Maschauer, D., Hofko, B. and Grothe, H. (2020). “Impact of reactive oxygen species on bitumen aging, The viennese binder aging method”, Construction and Building Materials, 257, 119495, https://doi.org/10.1016/j.conbuildmat.2020.119495.
Miyamoto, A. and Ximenes, H.D.C. (2021). “Development of a road-condition assessment system and application to road maintenance decision-making”, Civil Engineering Infrastructures Journal, 54(2), 225-251, https://doi.org/10.22059/CEIJ.2021.294057.1642.
Muñoz Perez, S.P. and Onofre Maicelo, P.A.A. (2021). “Use of recycled asphalt as an aggregate for asphalt mixtures: literary review”, Innovative Infrastructure Solution, 6, 146, https://doi.org/10.1007/s41062-021-00516-x
Omairey, E.L., Gu, F. and Zhang, Y. (2021). “An equation-based multiphysics modelling framework for oxidative ageing of asphalt pavements”, Journal of Cleaner Production, 280, 124401, https://doi.org/10.1016/j.jclepro.2020.124401.
Omairey, E.L., Zhang, Y., Soenen, H. and Carbonneau, X. (2022). “Parametric analysis and field validations of oxidative ageing in asphalt pavements using multiphysics modelling approaches”, International Journal of Pavement Engineering, 24(2), 1-24, https://doi.org/10.1080/10298436.2021.2020267. 
Qian, Y.,  Guo, F., Leng, Z., Zhang, Y. and Yu, H. (2020). “Simulation of the field aging of asphalt binders in different reclaimed asphalt pavement (RAP) materials in Hong Kong through laboratory tests”, Construction and Building Materials, 265, 120651, https://doi.org/10.1016/j.conbuildmat.2020.120651.
Read, J. and Whiteoak, D. (2003) The shell bitumen handbook, Thomas Telford Publishing Ltd., London.
Singh, B. and Kumar, P. (2015). “Effect of modifiers on the ageing properties of bitumen: A review”, Proceedings of 3rd Conference of Transportation Research Group of India (3rd CTRG), Kolkata.
Sirin, O., Paul, D.K. and Kassem, E., (2018). “State of the art study on aging of asphalt mixtures and use of antioxidant additives”, Advances in Civil Engineering, Article ID 3428961, 18 pages, https://doi.org/10.1155/2018/3428961.
Steiner, D., Hofko, B. and Blab, R. (2020). “Introducing a nitrogen conditioning to separate oxidative from non-oxidative ageing effects of hot mix asphalt”, Road Materials and Pavement Design, 21(5), 1293-1311, https://doi.org/10.1080/14680629.2018.1548371
Sreeram, A., Masad, A., Sootodeh Nia, Z., Maschauer, D., Mirwald, J., Hofko, B. and Bhasin, A., (2021). “Accelerated aging of loose asphalt mixtures using ozone and other reactive oxygen species”, Construction and Building Materials, 307, 124975, https://doi.org/10.1016/j.conbuildmat.2021.124975.
Wang, F., Xiao, Y., Cui, P., Lin, J., Li, M. and Chen, Z. (2020). “Correlation of asphalt performance indicators and aging degrees: A review”, Construction and Building Materials, 250, 118824, https://doi.org/10.1016/j.conbuildmat.2020.118824.
Wang, Y.,  Leng, Z., Li, X. and Hu, C. (2018). “Cold recycling of reclaimed asphalt pavement towards improved engineering performance”, Journal of Cleaner Production, 171, 1031-1038, https://doi.org/10.1016/j.jclepro.2017.10.132.
Wang, H. and Derewecki, K. (2013). “Rheological properties of asphalt binder partially substituted with wood lignin”, Airfield and Highway Pavement Conference, LA, California, https://doi.org/10.1061/9780784413005.081.
Xu, M., Yi, J., Pei, Z., Feng, D., Huang, Y. and Yang, Y. (2017). “Generation and evolution mechanisms of pavement asphalt aging based on variations in surface structure and micromechanical characteristics with AFM”, Materials Today Communication, 12, 106-118, https://doi.org/10.1016/j.mtcomm.2017.07.006.
Zhang, D., Zhang, H. and Shi, C. (2017). “Investigation of aging performance of SBS modified asphalt with various aging methods”, Construction and Building Materials, 145, 445-451, https://doi.org/10.1016/j.conbuildmat.2017.04.055.
Zhao, Z.J., Xu, S., Wu, W.F., Yu, J.Y. and Wu, S.P. (2015). “The aging resistance of asphalt containing a compound of LDHs and antioxidant”, Petroleum Science and Technology, 33, 787-793, https://doi.org/10.1080/10916466.2015.1014965